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vulnerability medal, shackles of war, a useful trinket =) let's discuss everything, but probably simple items, not SETS, as written in the topic title. in general, I think Armageddon's Blade is the best, not only as a simple artifact, but also as art; the Grail belongs to the artifacts :) it's a super-useful item! books, spheres, and wings are very good, but I'm for Armageddon's Blade.
P.S.: in Haven, the Golden Arrow is a very useful item during sieges! and I think artifacts should be discussed by category. How can you compare, for example, Gloves of Speed and a Mage's Hat (which gives all spells of the 5th level)? I'm not sure....